Fulleranes: The Hydrogenated Fullerenes

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Fulleranes are a special class of carbon molecules derived from fullerenes whose double bonds are partially or at least theoretically fully saturated by hydrogen. The hydrogenation changes the chemical properties of fullerenes which can become susceptible to substitution reactions as opposed to addition reactions to the double bonds (present in common fullerenes). One of the most intriguing aspects of fulleranes is the fact that they have been thought to exist in the interstellar medium or even in certain circumstellar media. The reasoning is quite simple: if fullerenes can be formed in the interstellar or better in the circumstellar medium, then they should undergo a simple hydrogenation reaction because of the ubiquitous presence of hydrogen in the universe. There is therefore a need not only to synthesize fulleranes in order to study their properties but also to study their infrared and electronic absorption spectra. Such spectra are used in the search for these molecules in the interstellar medium and around certain promising carbon-rich stars. Many efforts have been made by chemists and chemical physicists to synthesize these molecules at different degrees of hydrogenation and to record their spectra. Thus, Fulleranes:The Hydrogenated Fullerenes presents the state of the art research, synthesis and properties of these molecules; astrophysicists and astrochemists detail their expectations regarding the presence of these molecules in space.

Fulleranes: The Hydrogenated Fullerenes is written for researchers, postgraduates, and advanced undergraduates in organic synthetic chemistry, physical chemistry, and astrophysics.

Author(s): Susana Iglesias-Groth, Franco Cataldo (auth.), Franco Cataldo, Susana Iglesias-Groth (eds.)
Series: Carbon Materials: Chemistry and Physics 2
Edition: 1
Publisher: Springer Netherlands
Year: 2010

Language: English
Pages: 350
Tags: Organic Chemistry; Astrophysics and Astroparticles; Physical Chemistry

Front Matter....Pages i-xiv
Fulleranes and Carbon Nanostructures in the Interstellar Medium....Pages 1-25
Infrared and Ultraviolet Spectra of Fulleranes: HREELS Studies and Implications for the Interstellar Medium....Pages 27-37
The Potential Role Played by the Fullerene-Like Structures of Interstellar Carbon Dust in the Formation of Molecular Hydrogen in Space....Pages 39-53
Thermodynamic Properties of Fullerene Hydrides C 60 H 2n and Equilibria of Their Reactions....Pages 55-83
Fulleranes by Direct Reaction with Hydrogen Gas at Elevated Conditions....Pages 85-103
Chemical Methods to Prepare [60]Fulleranes....Pages 105-125
Synthesis, Stability and Spectroscopy of Perdeuterofulleranes: C 60 D 36 and C 70 D 38 Evidences of Isotope Effects....Pages 127-148
Isotope Effect in the UV Photolysis of Hydrogenated and Perdeuterated Fulleranes....Pages 149-170
Characterization of Hydrogenated Fullerenes by NMR Spectroscopy....Pages 171-202
Low Temperature Infrared Spectroscopy of C 60 and C 70 Fullerenes and Fullerane C 60 H 18 ....Pages 203-223
High-Pressure Hydrogenated Carbon Nanostructures....Pages 225-250
Topological Modeling of C 60 H 36 Hydrides....Pages 251-272
Back Matter....Pages 273-278