This thesis provides the first successful study of jump diffusion processes in glasses on the atomic scale, utilizing a novel coherent technique. This new method, called atomic-scale X-ray Photon Correlation Spectroscopy or aXPCS, has only recently been proven to be able to capture diffusion processes with atomic resolution in crystal systems.
With this new toolkit for studying atomic diffusion in amorphous systems, new insight into basic processes in a wide range of technically relevant materials, like fast ionic conductors, can be obtained.
Author(s): Manuel Ross (auth.)
Series: Springer Theses
Edition: 1
Publisher: Springer International Publishing
Year: 2016
Language: English
Pages: XVIII, 111
Tags: Spectroscopy and Microscopy; Ceramics, Glass, Composites, Natural Methods; Condensed Matter Physics
Front Matter....Pages i-xviii
Introduction....Pages 1-12
Theory....Pages 13-36
Experimental....Pages 37-54
Data Analysis....Pages 55-65
Proof of Concept: Direct Observation of Atomic Diffusion in Glasses....Pages 67-80
Practical Application: Tailoring Fast Ionic Diffusion....Pages 81-97
Conclusion....Pages 99-101
Back Matter....Pages 103-111